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Nuclear quantum effects such as zero-point energy conservation, tunnelling, non-adiabaticity and coherence play an important role in many complex chemical systems of technological and biological importance. This Faraday Discussion brings together both computational and experimental researchers who are interested in developing and applying methods that can be used to understand the role of quantum effects in complex systems. This volume provides a useful resource for researchers focussed on "many-particle" systems, including liquids, solids, biological complexes, and nanoparticles.